Time-Resolved Holography with Photoelectrons

Y. Huismans; A Rouzée; A Gijsbertsen; J H Jungmann; A S Smolkowska; P S W M Logman; F Lépine; C. Cauchy; S Zamith; T Marchenko; Joost M. Bakker; G. Berden; B Redlich; A F G van Der Meer; H G Muller; W Vermin; K J Schafer; M Spanner; M Yu Ivanov; O Smirnova; D. Bauer; S V Popruzhenko; M J J Vrakking

doi:10.1126/science.1198450

Time-Resolved Holography with Photoelectrons

Y. Huismans, A Rouzée, A Gijsbertsen, J H Jungmann, A S Smolkowska, P S W M Logman, F Lépine, C. Cauchy, S Zamith, T Marchenko, Joost M. Bakker, G. Berden, B Redlich, A F G van Der Meer, H G Muller, W Vermin, K J Schafer, M Spanner, M Yu Ivanov, O SmirnovaD. Bauer, S V Popruzhenko, M J J Vrakking

Research output: Contribution to Journal › Article › Academic › peer-review

Abstract

Ionization is the dominant response of atoms and molecules to intense laser fields and is at the basis of several important techniques, such as the generation of attosecond pulses that allow to measure electron motion in real time. We present experiments where metastable xenon atoms are ionized by intense 7-micrometer laser pulses from a free electron laser. Holographic structures are observed that record underlying electron dynamics on a sub-laser cycle time scale, enabling photoelectron spectroscopy with a time resolution almost two orders of magnitude higher than the duration of the ionizing pulse.

Original language	English
Pages (from-to)	61-64
Number of pages	3
Journal	Science (New York, N.Y.)
Volume	331
Issue number	6013
DOIs	https://doi.org/10.1126/science.1198450
Publication status	Published - 7 Jan 2011

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Huismans, Y., Rouzée, A., Gijsbertsen, A., Jungmann, J. H., Smolkowska, A. S., Logman, P. S. W. M., Lépine, F., Cauchy, C., Zamith, S., Marchenko, T., Bakker, J. M., Berden, G., Redlich, B., van Der Meer, A. F. G., Muller, H. G., Vermin, W., Schafer, K. J., Spanner, M., Ivanov, M. Y., ... Vrakking, M. J. J. (2011). Time-Resolved Holography with Photoelectrons. Science (New York, N.Y.), 331(6013), 61-64. https://doi.org/10.1126/science.1198450

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title = "Time-Resolved Holography with Photoelectrons",

abstract = "Ionization is the dominant response of atoms and molecules to intense laser fields and is at the basis of several important techniques, such as the generation of attosecond pulses that allow to measure electron motion in real time. We present experiments where metastable xenon atoms are ionized by intense 7-micrometer laser pulses from a free electron laser. Holographic structures are observed that record underlying electron dynamics on a sub-laser cycle time scale, enabling photoelectron spectroscopy with a time resolution almost two orders of magnitude higher than the duration of the ionizing pulse.",

author = "Y. Huismans and A Rouz{\'e}e and A Gijsbertsen and Jungmann, {J H} and Smolkowska, {A S} and Logman, {P S W M} and F L{\'e}pine and C. Cauchy and S Zamith and T Marchenko and Bakker, {Joost M.} and G. Berden and B Redlich and {van Der Meer}, {A F G} and Muller, {H G} and W Vermin and Schafer, {K J} and M Spanner and Ivanov, {M Yu} and O Smirnova and D. Bauer and Popruzhenko, {S V} and Vrakking, {M J J}",

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doi = "10.1126/science.1198450",

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volume = "331",

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Huismans, Y, Rouzée, A, Gijsbertsen, A, Jungmann, JH, Smolkowska, AS, Logman, PSWM, Lépine, F, Cauchy, C, Zamith, S, Marchenko, T, Bakker, JM, Berden, G, Redlich, B, van Der Meer, AFG, Muller, HG, Vermin, W, Schafer, KJ, Spanner, M, Ivanov, MY, Smirnova, O, Bauer, D, Popruzhenko, SV & Vrakking, MJJ 2011, 'Time-Resolved Holography with Photoelectrons', Science (New York, N.Y.), vol. 331, no. 6013, pp. 61-64. https://doi.org/10.1126/science.1198450

TY - JOUR

T1 - Time-Resolved Holography with Photoelectrons

AU - Huismans, Y.

AU - Rouzée, A

AU - Gijsbertsen, A

AU - Jungmann, J H

AU - Smolkowska, A S

AU - Logman, P S W M

AU - Lépine, F

AU - Cauchy, C.

AU - Zamith, S

AU - Marchenko, T

AU - Bakker, Joost M.

AU - Berden, G.

AU - Redlich, B

AU - van Der Meer, A F G

AU - Muller, H G

AU - Vermin, W

AU - Schafer, K J

AU - Spanner, M

AU - Ivanov, M Yu

AU - Smirnova, O

AU - Bauer, D.

AU - Popruzhenko, S V

AU - Vrakking, M J J

PY - 2011/1/7

Y1 - 2011/1/7

N2 - Ionization is the dominant response of atoms and molecules to intense laser fields and is at the basis of several important techniques, such as the generation of attosecond pulses that allow to measure electron motion in real time. We present experiments where metastable xenon atoms are ionized by intense 7-micrometer laser pulses from a free electron laser. Holographic structures are observed that record underlying electron dynamics on a sub-laser cycle time scale, enabling photoelectron spectroscopy with a time resolution almost two orders of magnitude higher than the duration of the ionizing pulse.

AB - Ionization is the dominant response of atoms and molecules to intense laser fields and is at the basis of several important techniques, such as the generation of attosecond pulses that allow to measure electron motion in real time. We present experiments where metastable xenon atoms are ionized by intense 7-micrometer laser pulses from a free electron laser. Holographic structures are observed that record underlying electron dynamics on a sub-laser cycle time scale, enabling photoelectron spectroscopy with a time resolution almost two orders of magnitude higher than the duration of the ionizing pulse.

U2 - 10.1126/science.1198450

DO - 10.1126/science.1198450

M3 - Article

C2 - 21163963

SN - 1095-9203

VL - 331

SP - 61

EP - 64

JO - Science (New York, N.Y.)

JF - Science (New York, N.Y.)

IS - 6013

ER -

Time-Resolved Holography with Photoelectrons

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